Using New Outlook on Windows for personal email, calendar, and contact management
Unified inbox not yet supported in the new outlook.
Remove the gmail account - when it asks to delete from the app or everywhere, choose everywhere.
Next, close the new Outlook, open the Run command (Windows key + R) and type or paste this command line. Note, there is a space before the two dashes -- and yes, you use two dashes.
olk.exe --clearLocalState
This deletes your profile and when you open the new Outlook, you'll need to add your account. Add additional accounts from the Settings dialog.